I recommend using 64 slices of a short sample for granular stuff, because that way you can automatically cut the ‘grains’ at zero crossings which minimises the sharp clicking you tend to get with other methods.
LFOs set to start time are a good idea too for a bit of movment, and I think if you carefully line up 2 or more LFOs with custom waveshapes you could probably generate some even more advanced effects…
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