Regarding organic ambient, you might look at Substan from this forum: Substan music - #74 by substan
A synth + samples combo is the most logical/powerful combo here, regardless of the devices.
I would say either DT + DN or DT + ST, and you feel the need for more you can maybe replace the DT by an OT.
- ST + DT: the more immediate combo, super flexible
- DN + DT: more synthesis options (and polyphony if you require it), especially for experimental stuff
Along with the DT, you can grab a portable Zoom recorder and go recording nature in the wild for the organic samples.
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